Aykroyd is an English surname. Notable people with the surname include:
- Dan Aykroyd (born 1952), Canadian comedian, actor, screenwriter and musician; brother of Peter
- Harold Ackroyd VC MC (1877–1917), soldier and recipient of the Victoria Cross
- James P. Aykroyd (1810−1835), early American composer, music teacher, musician
- Peter Aykroyd (1955−2021), Canadian comedian, actor, screenwriter and musician; brother of Dan
- William Aykroyd, 1st Baronet OStJ (1865−1947), English woollen and carpet manufacturer